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Volume 63, Issue 2
  • ISSN: 2056-5135
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  • oa Designing Parameters of Surfactant-Free Electrochemical Sensors for Dopamine and Uric Acid on Nitrogen Doped Graphene Films

    Evaluating the correlation between the content of N-configurations and the sensing for electrochemically active molecules

  • Authors: Boitumelo J. Matsoso1, Tsenolo Lerotholi1, Neil J. Coville1 and Glenn Jones2
  • Affiliations: 1 DST-NRF Centre of Excellence in Strong Materials and The Molecular Sciences Institute, School of Chemistry, University of the WitwatersrandPrivate Bag 3, PO WITS, 2050South Africa 2 Johnson MattheyBlounts Court, Sonning Common, Reading, RG4 9NHUK
  • Source: Johnson Matthey Technology Review, Volume 63, Issue 2, Apr 2019, p. 76 - 88
  • DOI: https://doi.org/10.1595/205651319X15472048744138
    • Published online: 01 Jan 2019

Abstract

Electrochemistry studies on the derivatives of graphene have been in the forefront of chemical research in recent years. The large specific surface area, high electrical conductivity, fast electron transfer rate and excellent biocompatibility to biomolecules constitute a few of the underlying reasons for the extensive application of graphene derivatives in modern electrochemistry and related technologies. Much interest in graphene derivatives has been driven by the ease of intentional functionalisation of the carbon backbone of graphene with dopants, such as nitrogen. Doping enhances the electrical conductivity and biocompatibility of nitrogen-doped graphene (NGr) nanomaterials and aids in their potential applications in electrochemical sensing and spectroelectrochemical devices. Despite the application of NGr in electrochemical sensing devices, the major challenge for reproducible industrial application still lies in the use of surfactants and binders and the limited knowledge on the correlation between the N-configurations and the electrocatalytic performance of these NGr-based electrodes. Therefore, the purpose of this short review article is to highlight some recent progress on the application of NGr derivatives for electrochemical detection of biomarkers such as uric acid and dopamine. The paper will also illustrate design parameters for new surfactant-free two-dimensional (2D) N-doped graphene based electrochemical sensors with variable N-functionalities for the detection of dopamine and uric acid.

© Johnson Matthey
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Designing Parameters of Surfactant-Free Electrochemical Sensors for Dopamine and Uric Acid on Nitrogen Doped Graphene Films
Johnson Matthey Technology Review 63, 76 (2019); https://doi.org/10.1595/205651319X15472048744138
/content/journals/10.1595/205651319X15472048744138
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