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Volume 65, Issue 1
  • ISSN: 2056-5135
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  • oa Comprehensive Review on High Hydrogen Permselectivity of Palladium Based Membranes: Part I

    Research progress of concentration polarisation phenomena

  • Authors: Hasan Mohd Faizal1,2, Bemgba B. Nyakuma3, Mohd Rosdzimin Abdul Rahman4, Md. Mizanur Rahman5, N. B. Kamaruzaman5 and S. Syahrullail5
  • Affiliations: 1 Automotive Development Centre, School of Mechanical Engineering, Faculty of Engineering, Universiti Teknologi Malaysia81310 UTM Johor Bahru, JohorMalaysia 2 School of Mechanical Engineering, Faculty of Engineering, Universiti Teknologi Malaysia81310 UTM Johor Bahru, JohorMalaysia 3 School of Chemical and Energy Engineering, Faculty of Engineering, Universiti Teknologi Malaysia81310 Skudai, Johor BahruMalaysia 4 Department of Mechanical Engineering, Faculty of Engineering, Universiti Pertahanan Nasional Malaysia, Kem Sg. Besi57000, Kuala LumpurMalaysia 5 School of Mechanical Engineering, Faculty of Engineering, Universiti Teknologi Malaysia81310 UTM Johor Bahru, JohorMalaysia
  • Source: Johnson Matthey Technology Review, Volume 65, Issue 1, Jan 2021, p. 64 - 76
  • DOI: https://doi.org/10.1595/205651320X15814149544965
    • Published online: 01 Jan 2021

Abstract

Palladium based membranes are widely used for supplying ultra-high purity hydrogen to a polymer electrolyte fuel cell (PEFC) installed on small vehicles and various electronic devices. Compared to pressure swing adsorption (PSA), the use of palladium based membrane is more economical for small size (small capacity) applications. The transportation of hydrogen through a palladium based membrane is governed by Sieverts’ Law and quantified with Fick’s First Law. Since the 20th century, the fabrication of high-performance palladium based membrane for enhanced hydrogen recovery performance has become practical. However, along with the improvement in hydrogen recovery performance, concentration polarisation becomes unavoidable because hydrogen permeation flux starts to affect hydrogen concentration at the membrane surface. Various parametric studies have investigated the effects of membrane thickness, hydrogen molar fraction and total upstream and downstream pressures on concentration polarisation level. The influence of membrane temperature, permeability, type and number of species in the hydrogen mixture, diffusivity of the hydrogen mixture, system configurations and flow patterns are also reported and comprehensively reviewed in this paper. Part II will complete the presentation.

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Comprehensive Review on High Hydrogen Permselectivity of Palladium Based Membranes: Part I
Johnson Matthey Technology Review 65, 64 (2021); https://doi.org/10.1595/205651320X15814149544965
/content/journals/10.1595/205651320X15814149544965
/content/journals/10.1595/205651320X15814149544965
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