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Volume 65, Issue 2
  • ISSN: 2056-5135
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  • oa Critical Review of Platinum Group Metal-Free Materials for Water Electrolysis: Transition from the Laboratory to the Market

    Earth-abundant borides and phosphides as catalysts for sustainable hydrogen production

  • Authors: Alexey Serov1, Kirill Kovnir2,3, Michael Shatruk4,5 and Yury V. Kolen’ko6
  • Affiliations: 1 Pajarito PowderLLC, Albuquerque, New Mexico 87109USA 2 Department of Chemistry, Iowa State UniversityAmes, Iowa 50011USA 3 Ames Laboratory, US Department of EnergyAmes, Iowa 50011USA 4 Department of Chemistry and Biochemistry, Florida State UniversityTallahassee, Florida 32306USA 5 National High Magnetic Field LaboratoryTallahassee, Florida 32310USA 6 International Iberian Nanotechnology LaboratoryBraga 4715-330Portugal
  • Source: Johnson Matthey Technology Review, Volume 65, Issue 2, Apr 2021, p. 207 - 226
  • DOI: https://doi.org/10.1595/205651321X16067419458185
    • Published online: 01 Jan 2021

Abstract

To combat the global problem of carbon dioxide emissions, hydrogen is the desired energy vector for the transition to environmentally benign fuel cell power. Water electrolysis (WE) is the major technology for sustainable hydrogen production. Despite the use of renewable solar and wind power as sources of electricity, one of the main barriers for the widespread implementation of WE is the scarcity and high cost of platinum group metals (pgms) that are used to catalyse the cathodic hydrogen evolution reaction (HER) and the anodic oxygen evolution reaction (OER). Hence, the critical pgm-based catalysts must be replaced with more sustainable alternatives for WE technologies to become commercially viable. This critical review describes the state-of-the-art pgm-free materials used in the WE application, with a major focus on phosphides and borides. Several emerging classes of HER and OER catalysts are reviewed and detailed structure–property correlations are comprehensively summarised. The influence of the crystallographic and electronic structures, morphology and bulk and surface chemistry of the catalysts on the activity towards OER and HER is discussed.

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2021-01-01
2024-12-26
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/content/journals/10.1595/205651321X16067419458185
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Critical Review of Platinum Group Metal-Free Materials for Water Electrolysis: Transition from the Laboratory to the Market
Johnson Matthey Technology Review 65, 207 (2021); https://doi.org/10.1595/205651321X16067419458185
/content/journals/10.1595/205651321X16067419458185
/content/journals/10.1595/205651321X16067419458185
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