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Volume 70, Issue 2
  • ISSN: 2056-5135
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Abstract

Single-atom catalysts (SACs) and single-atom alloy (SAA) catalysts are emerging as promising catalysts that allow maximising atom efficiency whilst improving catalyst performance. This literature review focuses on the evaluation of SACs and SAAs for thermocatalytic carbon dioxide methanation, providing mechanistic insights into carbon dioxide methanation on SACs and SAAs. The key findings from this review demonstrate that metal clusters (for example nickel and ruthenium) in many cases provide a greater catalytic efficiency on a metal loading basis for carbon dioxide methanation compared to SACs. In contrast, SAAs have demonstrated a notable positive effect on catalyst activity or selectivity for carbon dioxide methanation, with studies having identified the benefit of a SAA structure in providing these enhancements. Therefore, the use of either supported metal clusters (rather than single atoms) or SAAs shows the most potential in maximising metal atom efficiency in thermocatalytic carbon dioxide methanation.

© 2026 Johnson Matthey
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Comparative Analysis of Single-Atom Catalysts and Single-Atom Alloy Catalysts for Carbon Dioxide Methanation
Johnson Matthey Technology Review 70, 192 (2026); https://doi.org/10.1595/205651326X17557742534488
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